Un‐buc″kle (?), v. t. [1st pref. un- + buckle.] To loose the buckles of; to unfasten; as, to unbuckle a shoe. “Unbuckle anon thy purse.” Chaucer.
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Webster's Dictionary 1913
Webster's Revised Unabridged Dictionary, C. & G. Merriam Co., 1913.